Should the 'surfaces' tick box work automatically for molecules you draw in the workspace or do you have other tasks to complete before this works? One other question. I work as a chemistry teacher and saw a wonderful demo of Avogadro generating molecular orbitals in stunning detail. I don't have access to Gaussian. Is there any other way to generate these orbitals? Perhaps a database of molecules exist that can be imported to Avogadro. If so, how do I do this. Avogadro seems like a wonderful molecular viewer.
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