http://adsabs.harvard.edu/abs/2015EGUGA..17.2532M

On the feasibility of cirrus cloud thinning: Dependence of homo- and
heterogeneous ice nucleation on latitude and season

Authors:
Mitchell, David; Garnier, Anne; Avery, Melody

EGU General Assembly 2015, held 12-17 April, 2015 in Vienna, Austria.
id.2532
04/2015

Abstract

While GCM testing of cirrus cloud climate engineering (CE) reveals some
advantages over stratospheric aerosol injection, cirrus CE will not work
when ice is primarily formed through heterogeneous nucleation for T <
-38°C. Field campaigns have shown that ice in cold cirrus is generally
produced heterogeneously, but these campaigns have not addressed the cirrus
at high latitudes that would determine the effectiveness of cirrus CE. This
presentation introduces a new understanding of the satellite retrieved
"effective absorption optical depth ratio", or βeff, based on the 12.05 and
10.60 μm channels of the imaging infrared radiometer (IIR) aboard the
CALIPSO satellite. Using βeff calculations from in situ data, it is found
that βeff is tightly related to the N/IWC ratio, where N = ice particle
number concentration and IWC = ice water content. This is because N is
primarily determined by the smallest ice particles, and βeff is primarily
due to differences in wave resonance (i.e. photon tunneling) absorption, a
process that is only significant when ice particle maximum dimension D < ~
60 μm (i.e. when wavelength and effective particle size are comparable).
Thus βeff is a measure of the concentration of small (D < 60 μm) ice
crystals relative to the concentration of larger ice particles. Since
homogeneous ice nucleation generally results in N > 500 liter-1, with a
relatively high concentration of small ice crystals, βeff may be used to
determine when homogeneous nucleation dominates in a region for T < -38°C.
Satellite retrievals of βeff from anvil cirrus having N > 500 liter-1
(based on co-located/coincident in situ measurements) suggest that
homogeneous nucleation dominates when βeff > 1.15 ± 0.05. A global analysis
of βeff was conducted for the boreal summer (July-Aug.) and winter
(Jan.-Feb.) of 2007 and 2008, respectively. Using βeff to discriminate
between regions of homo- and heterogeneous ice nucleation for cirrus clouds
having emissivities between 0.4 and 0.7 and T < -38°C, our preliminary
results suggest that homogeneous ice nucleation is very common during the
winter months at high latitudes. This is consistent with GCM predicted
concentrations of mineral dust at 200 hPa, which are minimal during winter
at high latitudes. Regarding cirrus CE, it was recently shown that seeding
only 15% of the globe with the highest solar noon zenith angles at any
given time (i.e. the high latitudes during late fall-winter-spring)
produced a mean global cooling of 1.4°K, with much stronger cooling at high
latitudes. Our preliminary findings suggest that homogeneous ice nucleation
may dominate in winter at high latitudes, a necessary condition for this
seeding strategy to be viable.

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