https://www.atmos-chem-phys-discuss.net/acp-2017-722/

 

Kleinschmitt, Christoph; Boucher, Olivier; Platt, Ulrich (2017): Sensitivity of 
the radiative forcing by stratospheric sulfur geoengineering to the amount and 
strategy of the SO2 injection studied with the LMDZ-S3A model. In Atmos. Chem. 
Phys. Discuss., pp. 1–34. DOI: 10.5194/acp-2017-722.

 

Abstract. The enhancement of the stratospheric sulfate aerosol layer has been 
proposed as a method of geoengineering to abate global warming. Previous 
modelling studies found that stratospheric aerosol injection could effectively 
compensate the warming by greenhouse gases on the global scale, but also that 
the achievable cooling effect per sulfur mass unit, i.e. the forcing 
efficiency, decreases with increasing injection rate. In this study we use the 
atmospheric general circulation model LMDZ with the sectional aerosol module 
S3A to determine how the forcing efficiency depends on the injected amount, the 
injection height and the spatio-temporal pattern of injection. We find that the 
forcing efficiency may decrease more drastically for larger SO2 injections than 
previously estimated. As a result, the net instantaneous radiative forcing does 
not exceed −2 W m−2 for continuous equatorial injections and it decreases (in 
absolute value) for the largest injection rates simulated (50 Tg S yr−1). In 
contrast to other studies, the net radiative forcing in our experiments is 
fairly constant with injection height (in a range 17 to 23 km) for a given 
amount of SO2 injected. Also spreading the SO2 injections between 30 °S and 30 
°N or injecting only seasonally from varying latitudes does not result in a 
significantly larger (i.e. more negative) radiative forcing. Other key 
characteristics of our simulations include a consequent stratospheric heating 
caused by absorption of solar and infrared radiation by the aerosol, changes in 
stratospheric dynamics, with a collapse of the quasi-biennial oscillation at 
larger injection rates, which has impacts on the resulting spatial aerosol 
distribution, size and optical properties.

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