Hi All

If higher altitudes give longer life and so lower spray quantities they also  give a slower frequency response, longer phase lag and a greater chance of being stuck with what you do not want such as reflecting energy back down during Arctic winters as pointed out by Jan-Egil Kristjansson.

Advocates for marine cloud brightening are pleased about the short life of spray to give a high frequency response and the ability to stop Arctic cooling in the autumn before, it too, works the wrong way.

Stephen


Emeritus Professor of Engineering Design. School of Engineering, University of Edinburgh, Mayfield Road, Edinburgh EH9 3DW, Scotland s.sal...@ed.ac.uk, Tel +44 (0)131 650 5704, Cell 07795 203 195, WWW.homepages.ed.ac.uk/shs, YouTube Jamie Taylor Power for Change
On 17/12/2019 12:36, Andrew Lockley wrote:
Considering all effects, what's your view on the ideal height?

Andrew

On Tue, 17 Dec 2019, 08:47 Govindasamy Bala, <bala....@gmail.com <mailto:bala....@gmail.com>> wrote:

    26 km is probably not going to add any more benefit compared 25 km
    if you consider the effect identified in our paper but it is
    better when sedimentation effect is considered. More experiments
    with the NCAR WACCM model would be good to precisely nail this down.

    On Tue, Dec 17, 2019 at 2:10 PM Andrew Lockley
    <andrew.lock...@gmail.com <mailto:andrew.lock...@gmail.com>> wrote:

        Is 26k less good than 25?

        On Tue, 17 Dec 2019, 08:37 Govindasamy Bala,
        <bala....@gmail.com <mailto:bala....@gmail.com>> wrote:

            Andrew,

            Sedimentation effect works in the same direction as the
            effect we identified in our study. Therefore, higher the
            altitude of injection, the better. My judgement: 25 km
            would be good.

            On Mon, Dec 16, 2019 at 8:54 PM Andrew Lockley
            <andrew.lock...@gmail.com
            <mailto:andrew.lock...@gmail.com>> wrote:

                So what's your judgement on the ideal injection altitude?

                Andrew

                On Mon, 16 Dec 2019, 10:36 Govindasamy Bala,
                <bala....@gmail.com <mailto:bala....@gmail.com>> wrote:

                    Andrew,
                    Many modeling groups (e.g. Tilmes and others) have
                    already performed simulations that inject aerosols
                    at different heights and thus have included the
                    sedimentation effects and many many other effects.
                    These studies simulate the NET effects and hence
                    hard to interpret and quantify the individual
                    effects. The strength of our ESD paper is that it
                    changes only one variable and identifies its
                    individual contribution to the total problem.

                    What we have learnt during the course is that
                    there are too many variables in the aerosol SRM
                    problem (transport, location of injection,
                    aerosol-cloud interaction, aerosol-radiation
                    interaction, aerosol micro physics and the
                    resulting size distribution of the aerosols, etc.)
                    and the resulting uncertainties could be too
                    large. This is of course known to many of us for a
                    long time......

                    On Mon, Dec 16, 2019 at 3:41 PM Andrew Lockley
                    <andrew.lock...@gmail.com
                    <mailto:andrew.lock...@gmail.com>> wrote:

                        If I understand from the email below , you
                        used aerosols with no fall speed. Are
                        experiments planned to simulate aerosol descent?

                        Andrew

                        On Mon, 16 Dec 2019, 05:43 Govindasamy Bala,
                        <bala....@gmail.com
                        <mailto:bala....@gmail.com>> wrote:

                            Andrews,

                            We did not do experiments with aerosols
                            above 22 km. It is likely that the cooling
                            effect will be larger when aerosols are at
                            25 km. Beyond that it is likely that the
                            additional cooling benefits disappear. We
                            need more experiments to confirm this.

                            The sensitivity to height in our paper
                            arises mainly because of the increases in
                            stratospheric water vapor (which partly
                            offsets the cooling efficiency of the
                            aerosols) that is associated with the
                            stratospheric heating by the aerosols.
                            This increase in stratospheric water vapor
                            is largest when the aerosols (and the
                            heating) is close to the tropopause.

                            In our paper, we have isolated the effect
                            of just one factor. As Doug has pointed
                            out, the sedimentation effect would also
                            lead to more cooling if aerosols are
                            injected at higher altitudes...

                            Best,
                            Bala

                            On Sun, Dec 15, 2019 at 9:05 PM Douglas
                            MacMartin <dgm...@cornell.edu
                            <mailto:dgm...@cornell.edu>> wrote:

                                This is a great study to understand
                                the effectiveness per unit mass **in
                                the stratosphere**. Also keep in mind
                                that there’s an additional factor,
                                that at lower altitudes it takes
                                higher injection rates to achieve the
                                same burden in the stratosphere (i.e.,
                                lower lifetime at lower injected
                                altitude).

                                If the only thing you cared about was
                                cost, then since there are existing
                                studies demonstrating that you can
                                design an aircraft to get to ~20-21km,
                                we roughly know that it could be done,
                                but higher altitude injection means
                                less total sulfur injected and hence
                                smaller side effects, and should be
                                better understood both on the modeling
                                and implementation cost as the trade
                                may well be worth it.

                                doug

                                *From:*geoengineering@googlegroups.com
                                <mailto:geoengineering@googlegroups.com>
                                <geoengineering@googlegroups.com
                                <mailto:geoengineering@googlegroups.com>>
                                *On Behalf Of *Govindasamy Bala
                                *Sent:* Saturday, December 14, 2019
                                9:38 PM
                                *To:* Andrew Lockley
                                <andrew.lock...@gmail.com
                                <mailto:andrew.lock...@gmail.com>>
                                *Cc:* geoengineering
                                <geoengineering@googlegroups.com
                                <mailto:geoengineering@googlegroups.com>>
                                *Subject:* Re: [geo] Climate system
                                response to stratospheric sulfate
                                aerosols: sensitivity to altitude of
                                aerosol layer

                                Dear Andrew,

                                Thanks for the posting. The heights
                                studied were 16, 19 and 22 km, height
                                that are relevant to solar radiation
                                modification problem.. The final
                                paragraph in the paper is worth
                                reading to get more quantitative
                                information from this modeling study.

                                "To summarize, for the same mass, the
                                efficiency (defined

                                as changes in surface temperature per
                                Tg S) of volcanic
                                aerosol is less when it is prescribed
                                at lower altitudes in the
                                stratosphere (Fig. 9). For example, in
                                our simulations, there is
                                a surface cooling of 0.44K for each
                                teragram of sulfur placed
                                in the stratosphere at about 16 km
                                altitude (100 hPa). There
                                is an additional surface cooling of
                                0.15K per Tg S when the
                                prescribed altitude is increased from
                                about 16 km to about
                                22 km (37 hPa)."

                                On Sat, Dec 14, 2019 at 12:55 AM
                                Andrew Lockley
                                <andrew.lock...@gmail.com
                                <mailto:andrew.lock...@gmail.com>> wrote:

                                    Poster's note : this has
                                    significant implications for the
                                    engineering of delivery systems. I
                                    can't do the pressure altitude
                                    conversion in my head, but it's a
                                    lot higher than what's generally
                                    been planned for. We're gonna need
                                    a bigger boat.

                                    
https://www.earth-syst-dynam.net/10/885/2019/

                                    Climate system response to
                                    stratospheric sulfate aerosols:
                                    sensitivity to altitude of aerosol
                                    layer

                                    *Krishna-Pillai Sukumara-Pillai
                                    Krishnamohan et al. *Received: 01
                                    May 2019 – Discussion started: 23
                                    May 2019 – Revised: 24 Oct
                                    2019 – Accepted: 08 Nov
                                    2019 – Published: 13 Dec 2019

                                    Abstract

                                    top
                                    
<https://www.earth-syst-dynam.net/10/885/2019/#top>

                                    Reduction of surface temperatures
                                    of the planet by injecting sulfate
                                    aerosols in the stratosphere has
                                    been suggested as an option to
                                    reduce the amount of human-induced
                                    climate warming. Several previous
                                    studies have shown that for a
                                    specified amount of injection,
                                    aerosols injected at a higher
                                    altitude in the stratosphere would
                                    produce more cooling because
                                    aerosol sedimentation would take
                                    longer. In this study, we isolate
                                    and assess the sensitivity of
                                    stratospheric aerosol radiative
                                    forcing and the resulting climate
                                    change to the altitude of the
                                    aerosol layer. We study this by
                                    prescribing a specified amount of
                                    sulfate aerosols, of a size
                                    typical of what is produced by
                                    volcanoes, distributed uniformly
                                    at different levels in the
                                    stratosphere. We find that
                                    stratospheric sulfate aerosols are
                                    more effective in cooling climate
                                    when they reside higher in the
                                    stratosphere. We explain this
                                    sensitivity in terms of effective
                                    radiative forcing: volcanic
                                    aerosols heat the stratospheric
                                    layers where they reside, altering
                                    stratospheric water vapor content,
                                    tropospheric stability, and
                                    clouds, and consequently the
                                    effective radiative forcing. We
                                    show that the magnitude of the
                                    effective radiative forcing is
                                    larger when aerosols are
                                    prescribed at higher altitudes and
                                    the differences in radiative
                                    forcing due to fast adjustment
                                    processes can account for a
                                    substantial part of the dependence
                                    of the amount of cooling on
                                    aerosol altitude. These altitude
                                    effects would be additional to
                                    dependences on aerosol
                                    microphysics, transport, and
                                    sedimentation, which are outside
                                    the scope of this study. The
                                    cooling effectiveness of
                                    stratospheric sulfate aerosols
                                    likely increases with the altitude
                                    of the aerosol layer both because
                                    aerosols higher in the
                                    stratosphere have larger effective
                                    radiative forcing and because they
                                    have higher stratospheric
                                    residence time; these two effects
                                    are likely to be of comparable
                                    importance.

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                                With Best Wishes,

                                
-------------------------------------------------------------------
                                G. Bala
                                Professor
                                Center for Atmospheric and Oceanic
                                Sciences
                                Indian Institute of Science
                                Bangalore - 560 012
                                India

                                Tel: +91 80 2293 3428; +91 80 2293 2505
                                Fax: +91 80 2360 0865; +91 80 2293 3425
                                Email: gb...@iisc.ac.in
                                <mailto:gb...@iisc.ac.in>; bala.gov
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-- With Best Wishes,

                            
-------------------------------------------------------------------
                            G. Bala
                            Professor
                            Center for Atmospheric and Oceanic Sciences
                            Indian Institute of Science
                            Bangalore - 560 012
                            India

                            Tel: +91 80 2293 3428; +91 80 2293 2505
                            Fax: +91 80 2360 0865; +91 80 2293 3425
                            Email: gb...@iisc.ac.in
                            <mailto:gb...@iisc.ac.in>; bala.gov
                            <http://bala.gov>@gmail.com <http://gmail.com>
                            
Web:http://dccc.iisc.ac.in/dr_govindasamy_bala_profile.html
                            
-------------------------------------------------------------------



-- With Best Wishes,

                    
-------------------------------------------------------------------
                    G. Bala
                    Professor
                    Center for Atmospheric and Oceanic Sciences
                    Indian Institute of Science
                    Bangalore - 560 012
                    India

                    Tel: +91 80 2293 3428; +91 80 2293 2505
                    Fax: +91 80 2360 0865; +91 80 2293 3425
                    Email: gb...@iisc.ac.in <mailto:gb...@iisc.ac.in>;
                    bala.gov <http://bala.gov>@gmail.com
                    <http://gmail.com>
                    Web:http://dccc.iisc.ac.in/dr_govindasamy_bala_profile.html
                    
-------------------------------------------------------------------



-- With Best Wishes,

            -------------------------------------------------------------------
            G. Bala
            Professor
            Center for Atmospheric and Oceanic Sciences
            Indian Institute of Science
            Bangalore - 560 012
            India

            Tel: +91 80 2293 3428; +91 80 2293 2505
            Fax: +91 80 2360 0865; +91 80 2293 3425
            Email: gb...@iisc.ac.in <mailto:gb...@iisc.ac.in>;
            bala.gov <http://bala.gov>@gmail.com <http://gmail.com>
            Web:http://dccc.iisc.ac.in/dr_govindasamy_bala_profile.html
            -------------------------------------------------------------------



-- With Best Wishes,

    -------------------------------------------------------------------
    G. Bala
    Professor
    Center for Atmospheric and Oceanic Sciences
    Indian Institute of Science
    Bangalore - 560 012
    India

    Tel: +91 80 2293 3428; +91 80 2293 2505
    Fax: +91 80 2360 0865; +91 80 2293 3425
    Email: gb...@iisc.ac.in <mailto:gb...@iisc.ac.in>; bala.gov
    <http://bala.gov>@gmail.com <http://gmail.com>
    Web:http://dccc.iisc.ac.in/dr_govindasamy_bala_profile.html
    -------------------------------------------------------------------

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