https://egusphere.copernicus.org/preprints/2023/egusphere-2023-1983/

*Authors*
Christof Gerhard Beer, Johannes Hendricks, and Mattia Righi

*Citations*: Beer, C. G., Hendricks, J., and Righi, M.: Impacts of
ice-nucleating particles on cirrus clouds and radiation derived from global
model simulations with MADE3 in EMAC, EGUsphere [preprint],
https://doi.org/10.5194/egusphere-2023-1983, 2023.

*Received: 30 Aug 2023 – Discussion started: 04 Sep 2023*

*Abstract*. Atmospheric aerosols can act as ice-nucleating particles (INPs)
and influence the formation and the microphysical properties of cirrus
clouds, resulting in distinct climate effects. We employ a global
aerosol–climate model, including a two-moment cloud microphysical scheme
and a parametrization for aerosol-induced ice formation in cirrus clouds,
to quantify the climate impact of INPs on cirrus clouds. The model
considers mineral dust, (aviation) soot, crystalline ammonium sulfate, and
glassy organics as INPs in the cirrus regime. A number of sensitivity
experiments are performed to analyse various aspects of the simulated
INP-cirrus effect regarding (i) the ice-nucleating potential of the INPs,
(ii) the inclusion of ammonium sulfate and organic particles as INPs in the
model, and (iii) the model representations of vertical updrafts. The
resulting global radiative forcing of the total INP-cirrus effect,
considering all different INP-types, assuming a smaller and a larger ice
nucleating potential of INPs, is simulated as −28 and −55 mW m−2,
respectively. While the simulated impact of glassy organic INPs is mostly
small and not statistically significant, ammonium sulfate INPs contribute a
considerable radiative forcing, which is nearly as large as the combined
effect of mineral dust and soot INPs. Additionally, the anthropogenic
INP-cirrus effect is analysed considering the difference between
present-day (2014) and pre-industrial conditions (1750) and amounts to −29
mW m−2. In an additional sensitivity experiment we analyse the effect of
highly efficient INPs proposed for cirrus cloud seeding as a means to
reduce global warming by climate engineering. However, the results indicate
that this approach risks an overseeding of cirrus clouds and often results
in positive radiative forcings. Idealized experiments with prescribed
vertical velocities highlight the crucial role of the model dynamics for
the simulated INP-cirrus effects, e.g. resulting forcings increase about
one order of magnitude when increasing the prescribed vertical velocity.
The large discrepancy in the magnitude of the simulated INP-cirrus effect
between different model studies emphasizes the need for future detailed
analyses and efforts to reduce this uncertainty and constrain the resulting
climate impact of INPs.

*Source: EGU Sphere*

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