Thanks for the basis input advice. I used the dzvp-dft-orb basis(midi! had dependency problems), and tried to do a state-averaged CASSCF after a B3LYP dft optimimization. The output is below (the input is echoed). It stops with a new error during the integral sort. I haven't seen the error before. I can't find the names of the modules in the manual. Oh user-list, tell me, what are outbck(sort1) and mxbuck?

-Seth Olsen
Biophysics, UIUC

 Primary working directories:    /u/s/seth/molpro
 Secondary working directories:  /u/s/seth/molpro

blaslib=hpblas_pa20_64
mxmblk=120 mxmbln=120 ncache= 43200 mindgm= 33 mindgv= 32 mindgc= 33 mindgl= 33 mindgr= 33 noblas=0 nroll=4 minvec=7
default implementation of scratch files=df


***,GFP zwitterion spe w/ 6-31G* on S0 at 6-31G/CAS(2/2) optimized geometry
gprint,orbitals,civector;
!print the orbitals
memory,100,m
!memory specification
FILE,1,pIBIc108s5.int,new
FILE,2,pIBIc108s5.wfn,new
PUNCH,pIBIc108s5.pun,new
!don't save the integrals
geomtyp=xyz
!define basis set
geometry={nosymm,noorient;angstrom;
21
p-iodo-bi.xyz
C .000000 .000000 .000000
C .000000 .000000 1.419595
C 1.260000 .000000 2.068371
C 2.427296 .000021 1.339388
C 2.388903 -.000314 -.051610
C 1.159640 -.000401 -.722244
C -1.240895 .000226 2.106161
C -1.495551 .000127 3.465721
N -.597390 -.000165 4.513141
C -1.298495 -.000209 5.587936
N -2.643522 .000143 5.365847
C -2.862114 .000479 3.995157
O -3.930933 .000837 3.443641
H -3.365900 .000179 6.048703
H -.891541 -.000461 6.578763
H -2.128857 .000279 1.499275
H 1.296904 .000212 3.138020
H 3.376713 .001227 1.847522
H 1.154713 -.000497 -1.795700
H -.942028 .000172 -.518313
I 3.945667 -.001005 -1.449090
} !define z matrix for GFP in angstroms
!& don't use symmetry nor re-orient the molecule
basis
spd,c,dzvp-dft-orb,,,;
spd,o,dzvp-dft-orb,,,;
spd,n,dzvp-dft-orb,,,;
s,h,dzvp-dft-orb,,,;
spd,i,dzvp-dft-orb,,,;
end


 df=[b3lyp]
 rks
 wf,142,1,0
 optg

 mcscf
 occ,74
 closed,66
 state,5
 weight,1,1,1,1,1
 natorb,2141.2


put,xyz,pIBI.xyz,new put,molden,pIBIc108s5.molden,orb,2141.2


--- 1


*** PROGRAM SYSTEM MOLPRO ***
Copyright, University of Birmingham, 1997


Version 2002.4 linked 12, Dec AM 2003


**********************************************************************************************************************************
LABEL * GFP ZWITTERION SPE W/ 6-31G* ON S0 AT 6-31G/CAS(2/2) OPTIMIZED GEOMETR
HP-UX-B.11.11/mesa109(9000/785) 64 bit version DATE: 16-Dec-03 TIME: 00:12:33
**********************************************************************************************************************************


Installed patches: blas5 cc_ifc chgfracfix cilssym drv2el_llmp2 ecp_parse
fitmos fitmos6 ga_avqz ibm64_gmainv linux_gmalloc linux_ia64
linuxconf linuxconf2 linuxtune molproc_cray molproc_ibm myrinetports
opt_linear_triatomic p3_mkl parse_ibm rccsd rilmp2g_5 rs2grad
t1diag_uccsd2 test_cfit
**********************************************************************************************************************************



Variable memory set to 100000000 words, buffer space 230000 words



Permanent file 1 pibic108s5.int assigned. Implementation=df Permanent file 2 pibic108s5.wfn assigned. Implementation=df


PUNCHFILE PIBIC108S5.PUN OPENED SETTING GEOMTYP = XYZ SETTING DF = B3LYP


Using spherical harmonics


 Library entry C      S DZVP-DFT-ORB         selected for orbital group  1
 Library entry C      P DZVP-DFT-ORB         selected for orbital group  1
 Library entry C      D DZVP-DFT-ORB         selected for orbital group  1
 Library entry N      S DZVP-DFT-ORB         selected for orbital group  2
 Library entry N      P DZVP-DFT-ORB         selected for orbital group  2
 Library entry N      D DZVP-DFT-ORB         selected for orbital group  2
 Library entry O      S DZVP-DFT-ORB         selected for orbital group  3
 Library entry O      P DZVP-DFT-ORB         selected for orbital group  3
 Library entry O      D DZVP-DFT-ORB         selected for orbital group  3
 Library entry H      S DZVP-DFT-ORB         selected for orbital group  4
 Library entry I      S DZVP-DFT-ORB         selected for orbital group  5
 Library entry I      P DZVP-DFT-ORB         selected for orbital group  5
 Library entry I      D DZVP-DFT-ORB         selected for orbital group  5

1PROGRAM * SEWARD (Integral evaluation for generally contracted gaussian basis sets) Author: Roland Lindh, 1990

Geometry written to block 1 of record 700


Point group C1




ATOMIC COORDINATES

NR ATOM CHARGE X Y Z

   1  C       6.00    0.000000000    0.000000000    0.000000000
   2  C       6.00    0.000000000    0.000000000    2.682645565
   3  C       6.00    2.381054746    0.000000000    3.908654433
   4  C       6.00    4.586924333    0.000039684    2.531076312
   5  C       6.00    4.514372083   -0.000593374   -0.097528758
   6  C       6.00    2.191401845   -0.000757780   -1.364843257
   7  C       6.00   -2.344951531    0.000427078    3.980067178
   8  C       6.00   -2.826181592    0.000239995    6.549263043
   9  C       6.00   -2.453799748   -0.000394953   10.559667882
  10  C       6.00   -5.408611208    0.000905179    7.549752011
  11  N       7.00   -1.128903408   -0.000311805    8.528599838
  12  N       7.00   -4.995532225    0.000270231   10.139980527
  13  O       8.00   -7.428386249    0.001581701    6.507537893
  14  H       1.00   -6.360628705    0.000338261   11.430391256
  15  H       1.00   -1.684768198   -0.000871164   12.432059414
  16  H       1.00   -4.022956399    0.000527234    2.833218932
  17  H       1.00    2.450793193    0.000400622    5.929997947
  18  H       1.00    6.381062312    0.002318694    3.491310338
  19  H       1.00    2.182091165   -0.000939194   -3.393380958
  20  H       1.00   -1.780174794    0.000325033   -0.979469546
  21  I      53.00    7.456229472   -0.001899175   -2.738383033

Bond lengths in Bohr (Angstrom)

1--2 2.682645565 1--6 2.581673825 1-20 2.031842266 2--3 2.678155979 2--7 2.679944161
(1.419595000) (1.366163052) (1.075204701) (1.417219213) (1.418165479)


3--4 2.600688777 3-17 2.022546220 4--5 2.629606215 4-18 2.034941194 5--6 2.646181549
(1.376225333) (1.070285445) (1.391527783) (1.076844583) (1.400299073)


5-21 3.953307211 6-19 2.028559076 6-21 5.441049785 7--8 2.613876393 7-16 2.032476629
(2.092000234) (1.073467311) (2.879279757) (1.383203919) (1.075540391)


8--9 4.027656342 8-10 2.769462284 8-11 2.607398643 9-11 2.424992312 9-12 2.576148657
(2.131344103) (1.465536432) (1.379776041) (1.283250761) (1.363239259)


9-15 2.024168916 10-12 2.622959857 10-13 2.272818062 12-14 1.878469658
(1.071144139) (1.388010681) (1.202723610) (0.994043406)


Bond angles

1--2--3 117.24401062 1--2--7 118.95500544 1--6--5 119.46960926 1--6-19 121.65239278

1--6-21 162.70658910 2--1--6 121.91536822 2--1-20 118.82001968 2--3--4 120.77097677

2--3-17 119.21999005 2--7--8 129.56401309 2--7-16 116.69397218 3--2--7 123.80098305

3--4--5 120.40398933 3--4-18 119.85899580 4--3-17 120.00903170 4--5--6 120.19604034

4--5-21 130.33275109 5--4-18 119.73699046 5--6-19 118.87799558 5--6-21 43.23697984

5-21--6 27.29181211 6--1-20 119.26461145 6--5-21 109.47120805 7--8--9 164.08606351

7--8-10 121.78644952 7--8-11 128.77795441 8--7-16 113.74201339 8--9-11 38.42194422

8--9-12 75.31907008 8--9-15 162.97591432 8-10-12 102.11644437 8-10-13 131.52859630

8-11--9 106.26994654 9--8-10 74.12748697 9--8-11 35.30810924 9-12-10 108.43699825

9-12-14 127.23500872 10--8-11 109.43559582 10-12-14 124.32799303 11--9-12 113.74101418

11--9-15 124.55397023 12--9-15 121.70501557 12-10-13 126.35495899 19--6-21 75.64101739

 NUCLEAR CHARGE:                  142
 NUMBER OF PRIMITIVE AOS:         539
 NUMBER OF SYMMETRY AOS:          517
 NUMBER OF CONTRACTIONS:          517   ( 517A   )
 NUMBER OF CORE ORBITALS:          36   (  36A   )
 NUMBER OF VALENCE ORBITALS:       63   (  63A   )


NUCLEAR REPULSION ENERGY 1189.77906875



Eigenvalues of metric


1 0.256E-05 0.432E-04 0.125E-03 0.287E-03 0.551E-03 0.653E-03 0.846E-03 0.906E-03


Contracted 2-electron integrals neglected if value below 1.0D-12 AO integral compression algorithm 1 Integral accuracy 1.0D-12

6489.637 MB (compressed) written to integral file ( 9.0%)


NUMBER OF SORTED TWO-ELECTRON INTEGRALS: 8965073656. BUFFER LENGTH: 32768
NUMBER OF SEGMENTS: 188 SEGMENT LENGTH: 47835871 RECORD LENGTH: 65536


 Memory used in sort:      47.93 MW
 ? Error
 ? mxbuck too small
 ? The problem occurs in outbck(sort1)

ERROR EXIT


**********************************************************************************************************************************
DATASETS * FILE NREC LENGTH (MB) RECORD NAMES
1 18 6502.50 500 600 700 960 900 950 1000 1100 1400 1410
VAR BASINP GEOM ABASIS SYMINP ZMAT BASIS S T V
1200 1210 1080 1600 129 1650 1290 1300
H0 H01 AOSYM SMH P2S MOLCAS ERI ERIS


              2       4        0.88       500      600      700     1000
                                          VAR    BASINP    GEOM     BASIS

              4       1      285.25      1350
                                         BUCK

PROGRAMS * RKS-SCF
CPU TIMES * 2288.08
REAL TIME * 39 MIN,12.19 SEC CPU TIME * 38 MIN, 8.26 SEC I/O TIME * 0 MIN, 0.54 SEC
DISK USED * 6.79 GB
**********************************************************************************************************************************




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