https://acp.copernicus.org/preprints/acp-2022-295/

Robust evidence for reversal in the aerosol effective climate forcing trend

Johannes Quaas, Hailing Jia, Chris Smith, Anna Lea Albright, Wenche Aas,
Nicolas Bellouin, Olivier Boucher, Marie Doutriaux-Boucher, Piers M.
Forster, Daniel Grosvenor, Stuart Jenkins, Zig Klimont, Norman G. Loeb,
Xiaoyan Ma, Vaishali Naik, Fabien Paulot, Philip Stier, Martin Wild, Gunnar
Myhre, and Michael Schulz

Abstract.
Anthropogenic aerosols exert a cooling influence that offsets part of the
greenhouse gas warming. Due to their short tropospheric lifetime of only up
to several days, the aerosol forcing responds quickly to emissions. Here we
present and discuss the evolution of the aerosol forcing since 2000. There
are multiple lines of evidence that allow to robustly conclude that the
anthropogenic aerosol effective radiative forcing – both aerosol-radiation
and aerosol-cloud interactions – has become globally less negative, i.e.
that the trend in aerosol effective radiative forcing changed sign from
negative to positive. Bottom-up inventories show that anthropogenic primary
aerosol and aerosol precursor emissions declined in most regions of the
world; observations related to aerosol burden show declining trends, in
particular of the fine-mode particles that make up most of the anthropogenic
aerosols; satellite retrievals of cloud droplet numbers show trends
consistent in sign, as do observations of top-of-atmosphere radiation.
Climate model results, including a revised set that is constrained by
observations of the ocean heat content evolution show a consistent sign and
magnitude for a positive forcing relative to 2000 due to reduced aerosol
effects. This reduction leads to an acceleration of the forcing of climate
change, i.e. an increase in forcing by 0.1 to 0.3 W m-2, up to 12 % of the
total climate forcing in 2019 compared to 1750 according to IPCC.

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