http://www.atmos-chem-phys-discuss.net/15/30043/2015/acpd-15-30043-2015.html

03 Nov 2015

Climatic impacts of stratospheric geoengineering with sulfate, black carbon
and titania injection

A. C. Jones, J. M. Haywood, and A. Jones

Abstract. In this paper, we examine the potential climatic effects of
geoengineering by sulfate, black carbon and titania injection against a
baseline RCP8.5 scenario. We use the HadGEM2-CCS model to simulate
scenarios in which the top-of-the-atmosphere radiative imbalance due to
rising greenhouse gas concentrations is offset by sufficient aerosol
injection throughout the 2020–2100 period. We find that the global-mean
temperature is effectively maintained at historical levels for the entirety
of the period for all 3 aerosol-injection scenarios, though there are a
wide range of side-effects which are discussed in detail. The most
prominent conclusion is that although the BC injection rate necessary to
produce an equivalent global mean temperature-response is much lower, the
severity of stratospheric temperature changes (> +70 °C) and precipitation
impacts effectively exclude BC from being a viable option for
geoengineering. Additionally, while it has been suggested that titania
would be an effective particle because of its high scattering efficiency,
it also efficiently absorbs solar ultraviolet radiation producing a
significant stratospheric warming (> +20 °C). As injection rates for
titania are close to those for sulfate, there appears little benefit of
using titania when compared to injection of sulfur dioxide, which has the
added benefit of being well modelled through extensive research that has
been carried out on naturally occurring explosive volcanic eruptions.

Citation: Jones, A. C., Haywood, J. M., and Jones, A.: Climatic impacts of
stratospheric geoengineering with sulfate, black carbon and titania
injection, Atmos. Chem. Phys. Discuss., 15, 30043-30079,
doi:10.5194/acpd-15-30043-2015, 2015.

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