Paul, likely your system is affected by
Bug #1124803 "NetworkManager doesn't respond to SIGTERM in daemon mode"

You can check if this bug is related to your problem
by the following commands
sudo initctl status ureadahead-other
sudo lsof | grep ureadahead

This issue assumes /var/log/upstart/ureadahead-other.log
open for writing.

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https://bugs.launchpad.net/bugs/1181528

Title:
  /etc/init.d/umountroot: 'mount / is busy' due to upstart log file

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