Try xmlValidateDocument/xmlValidateDocumentFinal (sorry, I have no idea what are the Delphi names):
http://xmlsoft.org/html/libxml-valid.html#xmlValidateDocument
If it does not work (I recall someone reported problems in libxml mailing list) then try xmlValidateDtd/xmlValidateDtdFinal (I believe Daniel suggested this):
http://xmlsoft.org/html/libxml-valid.html#xmlValidateDtd
However, I do not remember if it worked or not. And there might be a bug (may be closed) in libxml bugzilla about this. Probably it has more recent info.
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