You can indeed run ATA100 drives on a 33 bus but there will be almost no speed 
increase - the 8mb cache may help but not 
much.
I put a similar 7200rpm ATA100 drive in my slot-loader 350 iMac and there was almost 
no speed increase at all.
I timed booting up, starting various programs and various file searches - only some of 
the searches where slightly faster and 
that was probably because some info was still cached.

I would spend the money on RAM. The 512MB in my 350 iMac turned it into an excellent 
OSX machine - it has yet to crash. It 
is perfectly responsive even compared to the newest offerings as long as you keep to a 
few apps at once.

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