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>ScienceWeek BULLETIN - April 12, 2000
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>
>This is SW BULLETIN, a free publication published each Monday by
>the Editors of SCIENCE-WEEK, the weekly Email research digest.
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>Table of Contents of the current issue of ScienceWeek will be
>found near the end of this file.
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>
>This Week's Report:
>
>ON SINGLE-MOLECULE PHYSICS AND CHEMISTRY
>Only a few decades ago, most scientists believed that individual
>molecules would not come within the domain of experimental
>observations within their lifetime, if ever, and that the
>statistical ensemble properties of molecules were therefore the
>only properties of relevance. That view has now undergone a
>dramatic alteration as a consequence of technological advances,
>and there is much excitement evident in many laboratories over
>the prospects of single-molecule explorations in physics,
>chemistry, and biology.
>... ... C. Bai et al (4 authors at 3 installations, CN US)
>present a short review of recent work in single-molecule physics
>and chemistry, the authors making the following points:
>     1) The authors point out that when Richard Feynman (1918-
>1988) was bothered while looking through one of the first
>*scanning tunneling microscopes, he was upset to have been
>interrupted because seeing the images of singe atoms was a
>"religious experience". For many generations of scientists, the
>molecule was both the concrete ultimate entity upon which our
>understanding of the everyday world was based, and at the same
>time an elusive intellectual construct whose very existence could
>only be inferred circumstantially by experiments on macroscopic
>samples. Thus, seeing an individual atom or molecule in motion
>brings immediate emotional impact to this central concept of
>modern thought.
>     2) The authors ask: "When is molecular individuality
>important?" The new possibility of studying single molecules is
>important because molecular individuality does finally come into
>play when the molecule is a complex entity. This may occur
>because the molecule itself may have an intricate internal
>structure -- e.g., a biomolecule -- resulting in a complex energy
>landscape. Alternatively, the molecule may be part of a complex
>environment that substantially changes the behavior of the
>molecule. Here, distinguishing different molecules at different
>locales is crucial for understanding the system as a whole.
>Biomolecules in living cells are examples of this. Even simple
>inorganic molecules on structured surfaces or in disordered
>systems such as viscous liquids or glasses provide situations in
>which molecular individuality matters. In all of these cases, the
>capability of studying an individual molecule over time can
>provide new insights unavailable by straightforward experiments
>on macroscopic populations of molecules.
>     3) With the aid of *scanning probe microscopy, direct
>observations of entire arrays of atoms, molecules, and the fine
>structures of molecular aggregates have become possible. The
>ability to precisely control probes permits the study of long-
>range structures made by molecules lying on surfaces. However,
>although pretty pictures of such systems are easy to construct,
>obtaining quantitative characteristics of surface-bound molecules
>is not entirely straightforward, and the rigorous interpretation
>of scanning probe microscopy images requires substantial
>theoretical as well as experimental effort.
>     4) The authors conclude: "We are only at the beginning, but
>it is clear there is much to be discovered of a fundamental
>nature about complex molecules viewed as individuals. Perhaps
>equally important will be the idea of single molecule control.
>Now that experiments interact with molecules at an individual
>level, we can try to control them as individuals, not as
>populations. A molecule under active control by an adaptive
>environment will be a new beast. Such tamed molecules may well
>resemble much more the elegant engineered machinery of everyday
>experience than the unruly, wild molecules we are used to
>studying today."
>-----------
>C. Bai et al: Single molecule physics and chemistry.
>(Proc. Natl. Acad. Sci. US 28 Sep 99 96:11075)
>QY: Chunli Bai, Institute of Chemistry, The Chinese Academy of
>Sciences, Beijing 100080 CN.
>-----------
>Text Notes:
>... ... *scanning tunneling microscopes: First available in the
>early 1980s, this technique involves an atomically sharp metal
>tip brought in atomic proximity (e.g., 0.5 to 1 nanometer) to a
>flat surface so that electrons can *tunnel between the two
>systems. Recording the atomic modulation of the atomic structure
>which scanning the tip across the surface allows one to image
>adsorbed species and surface morphologies.
>... ... tunnel: Tunneling is a quantum mechanical phenomenon
>involving an effective penetration of an energy barrier resulting
>from the width of the barrier being less than the wavelength of
>the particle.
>... ... *scanning probe microscopy: A general term comprising all
>atomic-level probe techniques. See background material below.
>-------------------
>Summary & Notes by SCIENCE-WEEK [http://scienceweek.com] 3Dec99
>[For more information: http://scienceweek.com/swfr.htm]
>-------------------
>Related Background:
>ON THE NANOSCALE SCIENCE OF SINGLE MOLECULES
>In recent years, experiments on individual molecules using
>scanning probe microscopies [*Note #1] have demonstrated a
>diversity of physical, chemical, mechanical, and electronic
>phenomena. These techniques have permitted deeper insight into
>the quantum electronics of molecular systems and have provided
>unique information about the conformational and mechanical
>properties of these systems. Concomitant developments in
>experimentation and theory have allowed a diverse range of
>molecules to be studied, molecules varying in complexity from
>simple diatomic systems to biological macromolecular systems.
>... ... J.K. Gimzewski and C. Joachim (2 installations, CH FR)
>present an extensive review of current single-molecule research,
>the authors making the following points: 1) The very nature of
>proximal probe methods encourages exploration of the nanoworld
>beyond conventional microscopic imaging. Scanning probes now
>allow us to perform "engineering" operations on single molecules,
>atoms, and bonds, thereby providing a tool that operates at the
>ultimate limits of fabrication. These techniques have also
>enabled explorations of molecular properties on an individual
>basis as opposed to explorations restricted to the statistical
>properties of large populations of molecules. 2) The
>nanomechanical properties of individual molecules take the form
>of vibrations, rotations, conformational changes, and
>translations. *Inelastic tunneling processes, probe-tip-induced
>forces, and Brownian motion have been found to drive mechanical
>responses in individual molecules, and these aspects are the
>focus of current research. The important role of thermal noise at
>room temperature in nanoscale systems suggests that future
>technologies for building small energy-efficient devices will
>need to use ambient temperature fluctuations rather than fight
>against them. 3) Future developments in single-molecule nanoscale
>science call for a close integration of chemistry, biology,
>physics, and technology in terms of synthesis, theoretical
>modeling, and advanced scanning probe microscope techniques.
>Although scanning probe microscopy has been shown to be an
>ultimate probe for investigating the properties of individual
>molecules, it is still an open question whether these techniques
>have the intrinsic capabilities to be useful fabrication tools in
>technology. The recent development of massive micromechanical
>arrays of thousands of scanning probe microscopy probes suggests
>that such a possibility is becoming more real each day.
>-----------
>J.K. Gimzewski and C. Joachim: Nanoscale science of single
>molecules using local probes.
>(Science 12 Mar 99 283:1683)
>QY: James K. Gimzewski [[EMAIL PROTECTED]]
>-----------
>Text Notes:
>... ... *Note #1: The general approach in scanning probe
>microscopy research is illustrated by consideration of two major
>techniques, scanning tunneling microscopy (STM) and atomic force
>microscopy (AFM). In scanning tunneling microscopy, an atomically
>sharp metal tip is brought in atomic proximity (e.g., 0.5 to 1
>nanometer) to a flat surface so that electrons can *tunnel
>between the two systems. The probe is slowly moved across the
>surface and raised and lowered so as to keep the tunneling
>current constant. A computer-generated contour map of the surface
>is thus produced. The technique can resolve individual atoms, but
>requires electrically conducting materials. In atomic force
>microscopy, a tip is fixed to a cantilever whose position is
>monitored while the tip scans the surface. The force between the
>tip and the surface determines the position of the cantilever.
>When recorded in atomic resolution, the image represents a map of
>atomic forces at the surface. The advantage of atomic force
>microscopy is that the probed surface does not need to be
>electrically conducting.
>... ... *tunnel: "Tunneling" is a quantum mechanical
>phenomenon involving an effective penetration of an energy
>barrier resulting from the width of the barrier being less than
>the wavelength of the particle.
>... ... *Inelastic tunneling processes: In general, an
>"inelastic" process is a process which results in a permanent
>change in the properties of a system. In this context, the term
>"inelastic tunneling process" refers to a technique involving the
>input of energy into a single-molecule system to selectively
>excite chemical bonds or to perform spectroscopic studies of the
>system.
>-------------------
>Summary & Notes by SCIENCE-WEEK [http://scienceweek.com] 21May99
>-------------------
>Related Background:
>ON REACTIONS ON SEMICONDUCTOR SURFACES
>Chemical reactions on surfaces are important in many areas of
>science and technology. On metal surfaces, the electronic states
>of the surface atoms are spatially extended and can therefore be
>easily shared with those of reactive species, the result a
>dramatic influence on the structure of these species as they
>approach the surface. In contrast, bonding on semiconductor
>surfaces is largely covalent, and surface electronic states tend
>to be spatially localized. ... ... Harry E. Ruda (University of
>Toronto, CA) presents a short review of current research
>concerning reactions on semiconductor surfaces, the author making
>the following points: 1) Understanding of the interactions of
>species with semiconductor surfaces has been considerably
>advanced by the widespread use of *scanning tunneling microscopy
>(STM), which can probe, with atomic resolution, the spatial
>extent of electron density on a surface. 2) Bias-dependent
>scanning tunneling microscopy studies, in which images are taken
>at different voltages between the STM tip and the sample, allow
>the determination of the energy spectra of surface electronic
>states, and in special cases enable discrimination between
>different chemical species. 3) Coupled with computer modeling,
>which can provide increasingly realistic descriptions of the
>pertinent underlying physics, scanning tunneling microscopy
>studies are providing  the information needed to understand and
>control the interactions of chemical species on semiconductor
>surfaces. The author concludes: "This research will have a
>profound influence on nanotechnology, slated to become the
>cornerstone of coming generations of semiconductor devices and
>circuitry."
>-----------
>Harry E. Ruda: Reactions on semiconductor surfaces.
>(Science 29 Jan 99 283:646)
>QY: Harry E. Ruda [[EMAIL PROTECTED]]
>-------------------
>Summary by SCIENCE-WEEK [http://scienceweek.com] 9Apr99
>[For more information: http://scienceweek.com/swfr.htm]
>
>[SW Bulletin 12 Apr 00]
>
>****************************************************************
>
>Contents of the Current Issue of ScienceWeek:
>
>April 14, 2000 -- Vol. 4 Number 15
>-----------------------------------------------
>1. Neurobiology:
>On the Biological Basis of Memory
>---------------------------------
>Although the idea that processes underlying new memories
>initially persist in a fragile state and then consolidate over
>time still guides research on memory, neurobiologists do not yet
>have a consensus theory concerning the biological basis of memory
>formation. (Includes related background material.)
>
>2. Neurobiology:
>Functional Regeneration of Sensory Axons in Adult Spinal Cord
>-------------------------------------------------------------
>Natural repair of severed connections between the spinal cord and
>spinal nerves does not occur in humans, but in the past decade
>there has been much progress in understanding the mechanisms of
>nerve fiber regeneration. There is now new evidence of functional
>regeneration of dorsal root sensory axons in adult mammalian
>spinal cord after treatment by local introduction of neurotrophic
>factors. (Includes related background material.)
>
>3. Medical Biology:
>On New Approaches to Human Aging
>--------------------------------
>The resolution of all causes of death currently written on the
>death certificates of those older than 65 will result only in an
>increase in life expectancy of approximately 15 years. Any major 
>increase in human life span will require knowledge of the
>fundamental biology of the aging process. (Includes related
>background material.)
>
>4. Earth Sciences:
>Ice-Core Evidence of Abrupt Climate Changes
>-------------------------------------------
>Records of abrupt changes in Earth's climate are particularly
>clear in high-resolution ice cores, which can preserve histories
>of local climate, regional climate, and broader climate -- all on
>a common time scale. (Includes related background material.)
>
>5. Astrobiology:
>Evidence for Sufficient Energy for a Biosphere on Europa
>--------------------------------------------------------
>Disequilibrium chemistry in the ice cover of Europa's oceans,
>driven by charged particles accelerated in Jupiter's
>magnetosphere, should produce enough organic and oxidant
>molecules to fuel a substantial Europan biosphere. (Includes
>related background material.)
>
>6. Astrophysics:
>On Stars, Brown Dwarfs, and Superplanets
>----------------------------------------
>As recently as 1994, brown dwarfs were "theoretical" stars, with
>no brown dwarfs considered to be unambiguously identified. During
>the past few years, dozens of brown dwarfs have been discovered,
>and it is now apparent they are as numerous as ordinary stars.
>(Includes related background material.)
>
>In Focus: On Carbon (Includes related background material.)
>
>Total text 86K ASCII bytes
>
>****************************************************************
>
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