The KEY to this effect is particle chirlity. Only left hand particles
decay.
http://www.nature.com/articles/524008b
Any mechanism that change the chirality of particles to left handed will
increase the rate at which these particles decay.
One mechanism that effects nuclear decay rates is surface
It sounds like that the pitchblende begins as a pretty good metal oxide
dielectric, and as the Purcell processing commences, some oxide is lost and
the sample becomes conductive. Once the sample becomes conductive, the
electric field is shorted out across the sample. This is also why it won't
wor
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