Ok, after escalating from random-questions-embedded-in-a-long-posting to open-conjecture-with-direct-questions and getting nowhere, I went with the shakily-supported-but-loudly-declared-claim-of-fact route so popular on the internet, and that elicited a couple of responses from kind and knowledgeable researchers (Merci!). Although I did not resolve all of the questions which formed the basis of my conjecture about a potential signal hidden within the noise of the peak-69 artifacts, I am able to infer and presume the following:
1) Although not directly specified, the sputter-cleaning ion source was most likely also isotopically-pure Ga-69. This and many other models of ToF-SIMS analyzers are apparently capable of performing sputter-cleaning and SIMS-scanning with a variety of ion sources, using either the same or different sources, notably including cesium, argon, oxygen, and gold. In this case, given only a single ion source specified, common practice implies that they are both performed with Ga69. 2) The high variability of residual Ga69 in different post-sputtering sample spectra (particularly figure 11b) is apparently within the normal variance range for different sample substances. So, if there is something interesting to be found regarding a mass-69 species, it will need to be discovered using an analytic method that does not employ Ga-69 such as this one does. I hope that other analytic results will be published soon! Unless and until then, I'll just presume this to be artifact. -Bob > From: Robert Ellefson > Sent: Tuesday, October 14, 2014 5:29 PM > Subject: [Vo]:Testing fuels without a reactor > > Given the results of the SIMS analysis from the Lugano report, particularly > as detailed in this posting: > http://www.mail-archive.com/vortex-l@eskimo.com/msg98596.html > > I believe that it is possible to evaluate the nuclear activity of candidate > fuel samples simply by sputter-cleaning them as part of a ToF-SIMS analysis. > If researchers with access to such analytic equipment were willing to run > the experiment, I believe that a successful replication of Rossi's reaction > can be observed occurring with before-and-after spectra of the fuel. > > So, skip the reactors, start evaluating powders in the SEM itself!